Foundations of Nonlinear Optical Microscopy
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Foundations of Nonlinear Optical Microscopy
Potma, Eric Olaf
John Wiley & Sons Inc
03/2024
448
Dura
Inglês
9781119814887
15 a 20 dias
666
Descrição não disponível.
Preface xiii
Acknowledgments xv
1 Light: Electromagnetic Radiation 1
1.1 Introduction 1
1.2 Electromagnetic Fields 1
1.3 Transverse Waves 7
1.4 Polarization States 15
1.5 Reflection and Transmission at Interfaces 19
1.6 Transformation of the Field by a Lens 23
1.7 Intensity and Energy 29
Bibliography 31
2 Focused Light 33
2.1 Introduction 33
2.2 Interference of Multiple Waves 34
2.3 The Scalar Focal Field 38
2.4 The Focused Vector Field 49
2.5 Aberrations 60
Bibliography 65
3 Ultrafast Pulses 67
3.1 Introduction 67
3.2 Optical Pulses in the Frequency Domain 68
3.3 Optical Pulses in the Time Domain 77
3.4 Measurement of Pulse Duration 88
3.5 Pulse Properties and Nonlinear Optical Signals 95
3.6 Noise 97
Bibliography 102
4 Classical Model of Nonlinear Optics 105
4.1 Introduction 105
4.2 Linear Optical Response 105
4.3 Nonlinear Optical Response 115
4.4 Properties of Nonlinear Susceptibilities 124
Bibliography 134
5 Semiclassical Model of Nonlinear Optics 137
5.1 Introduction 137
5.2 Quantum Mechanical Concepts 138
5.3 Density Matrix Formalism 147
5.4 Perturbation Expansion for the Density Matrix 152
5.5 Linear and Nonlinear Susceptibilities 159
5.6 Quantization of the Electromagnetic Field 164
Bibliography 172
6 Nonlinear Optical Signals: Molecular Transitions, Signal Radiation, Propagation, and Detection 175
6.1 Introduction 175
6.2 Molecular Transitions 175
6.3 Spatial Properties of Radiated Signal 187
6.4 Signal Radiation and Detection 205
Bibliography 211
7 Multiphoton Absorption and Fluorescence Microscopy 213
7.1 Introduction 213
7.2 Physics of Nonlinear Absorption 214
7.3 Optical Sectioning and Imaging Resolution 223
7.4 Direct Detection of Multiphoton Absorption 228
7.5 Fluorescence Detection of Multiphoton Absorption 232
Bibliography 241
8 Pump-Probe Microscopy 245
8.1 Introduction 245
8.2 Pump-Probe Signals in Microscopy 246
8.3 Electronic Pump-Probe Spectroscopy 250
8.4 Detection of Pump-Probe Signals 264
8.5 Imaging Based on the Photothermal Effect 269
Bibliography 277
9 Harmonic Generation Microscopy 281
9.1 Introduction 281
9.2 Molecular Response in Harmonic Imaging 282
9.3 SHG Imaging of Fibrillar Structures 292
9.4 THG Imaging of ?(3) Discontinuities 304
Bibliography 310
10 Sum-Frequency Generation Microscopy 313
10.1 Introduction 313
10.2 Molecular Vibrations 314
10.3 Molecular Vibrations in Sum-Frequency Generation 324
10.4 Collinear Sum-Frequency Generation Microscopy 334
10.5 Third-Order Sum-Frequency Generation Microscopy 344
Bibliography 348
11 Coherent Raman Scattering Microscopy 351
11.1 Introduction 351
11.2 The Raman Effect 353
11.3 Coherent Raman Scattering 359
11.4 Raman Spectroscopy of Lipids 373
11.5 Imaging Properties of CARS 378
11.6 Imaging Properties of SRS 387
11.7 Spectral Resolution 391
Bibliography 398
Appendix A Fourier Transform Relationships 401
Appendix B Wavenumbers Unit 403
Appendix C Power Spectral Density of White Noise 405
Appendix D Fermi's Golden Rule 407
Appendix E Population Dynamics with Relaxation 411
Appendix F Stimulated Raman Scattering with Quantized Fields 413
Index 415
Acknowledgments xv
1 Light: Electromagnetic Radiation 1
1.1 Introduction 1
1.2 Electromagnetic Fields 1
1.3 Transverse Waves 7
1.4 Polarization States 15
1.5 Reflection and Transmission at Interfaces 19
1.6 Transformation of the Field by a Lens 23
1.7 Intensity and Energy 29
Bibliography 31
2 Focused Light 33
2.1 Introduction 33
2.2 Interference of Multiple Waves 34
2.3 The Scalar Focal Field 38
2.4 The Focused Vector Field 49
2.5 Aberrations 60
Bibliography 65
3 Ultrafast Pulses 67
3.1 Introduction 67
3.2 Optical Pulses in the Frequency Domain 68
3.3 Optical Pulses in the Time Domain 77
3.4 Measurement of Pulse Duration 88
3.5 Pulse Properties and Nonlinear Optical Signals 95
3.6 Noise 97
Bibliography 102
4 Classical Model of Nonlinear Optics 105
4.1 Introduction 105
4.2 Linear Optical Response 105
4.3 Nonlinear Optical Response 115
4.4 Properties of Nonlinear Susceptibilities 124
Bibliography 134
5 Semiclassical Model of Nonlinear Optics 137
5.1 Introduction 137
5.2 Quantum Mechanical Concepts 138
5.3 Density Matrix Formalism 147
5.4 Perturbation Expansion for the Density Matrix 152
5.5 Linear and Nonlinear Susceptibilities 159
5.6 Quantization of the Electromagnetic Field 164
Bibliography 172
6 Nonlinear Optical Signals: Molecular Transitions, Signal Radiation, Propagation, and Detection 175
6.1 Introduction 175
6.2 Molecular Transitions 175
6.3 Spatial Properties of Radiated Signal 187
6.4 Signal Radiation and Detection 205
Bibliography 211
7 Multiphoton Absorption and Fluorescence Microscopy 213
7.1 Introduction 213
7.2 Physics of Nonlinear Absorption 214
7.3 Optical Sectioning and Imaging Resolution 223
7.4 Direct Detection of Multiphoton Absorption 228
7.5 Fluorescence Detection of Multiphoton Absorption 232
Bibliography 241
8 Pump-Probe Microscopy 245
8.1 Introduction 245
8.2 Pump-Probe Signals in Microscopy 246
8.3 Electronic Pump-Probe Spectroscopy 250
8.4 Detection of Pump-Probe Signals 264
8.5 Imaging Based on the Photothermal Effect 269
Bibliography 277
9 Harmonic Generation Microscopy 281
9.1 Introduction 281
9.2 Molecular Response in Harmonic Imaging 282
9.3 SHG Imaging of Fibrillar Structures 292
9.4 THG Imaging of ?(3) Discontinuities 304
Bibliography 310
10 Sum-Frequency Generation Microscopy 313
10.1 Introduction 313
10.2 Molecular Vibrations 314
10.3 Molecular Vibrations in Sum-Frequency Generation 324
10.4 Collinear Sum-Frequency Generation Microscopy 334
10.5 Third-Order Sum-Frequency Generation Microscopy 344
Bibliography 348
11 Coherent Raman Scattering Microscopy 351
11.1 Introduction 351
11.2 The Raman Effect 353
11.3 Coherent Raman Scattering 359
11.4 Raman Spectroscopy of Lipids 373
11.5 Imaging Properties of CARS 378
11.6 Imaging Properties of SRS 387
11.7 Spectral Resolution 391
Bibliography 398
Appendix A Fourier Transform Relationships 401
Appendix B Wavenumbers Unit 403
Appendix C Power Spectral Density of White Noise 405
Appendix D Fermi's Golden Rule 407
Appendix E Population Dynamics with Relaxation 411
Appendix F Stimulated Raman Scattering with Quantized Fields 413
Index 415
Este título pertence ao(s) assunto(s) indicados(s). Para ver outros títulos clique no assunto desejado.
Light propagation; focusing of light; pulses of light; light-matter interactions; molecular excitations; signal radiation; detection of light; multi-photon excited fluorescence; harmonic generation; sum-frequency generation; coherent Raman scattering; pump-probe microscopy
Preface xiii
Acknowledgments xv
1 Light: Electromagnetic Radiation 1
1.1 Introduction 1
1.2 Electromagnetic Fields 1
1.3 Transverse Waves 7
1.4 Polarization States 15
1.5 Reflection and Transmission at Interfaces 19
1.6 Transformation of the Field by a Lens 23
1.7 Intensity and Energy 29
Bibliography 31
2 Focused Light 33
2.1 Introduction 33
2.2 Interference of Multiple Waves 34
2.3 The Scalar Focal Field 38
2.4 The Focused Vector Field 49
2.5 Aberrations 60
Bibliography 65
3 Ultrafast Pulses 67
3.1 Introduction 67
3.2 Optical Pulses in the Frequency Domain 68
3.3 Optical Pulses in the Time Domain 77
3.4 Measurement of Pulse Duration 88
3.5 Pulse Properties and Nonlinear Optical Signals 95
3.6 Noise 97
Bibliography 102
4 Classical Model of Nonlinear Optics 105
4.1 Introduction 105
4.2 Linear Optical Response 105
4.3 Nonlinear Optical Response 115
4.4 Properties of Nonlinear Susceptibilities 124
Bibliography 134
5 Semiclassical Model of Nonlinear Optics 137
5.1 Introduction 137
5.2 Quantum Mechanical Concepts 138
5.3 Density Matrix Formalism 147
5.4 Perturbation Expansion for the Density Matrix 152
5.5 Linear and Nonlinear Susceptibilities 159
5.6 Quantization of the Electromagnetic Field 164
Bibliography 172
6 Nonlinear Optical Signals: Molecular Transitions, Signal Radiation, Propagation, and Detection 175
6.1 Introduction 175
6.2 Molecular Transitions 175
6.3 Spatial Properties of Radiated Signal 187
6.4 Signal Radiation and Detection 205
Bibliography 211
7 Multiphoton Absorption and Fluorescence Microscopy 213
7.1 Introduction 213
7.2 Physics of Nonlinear Absorption 214
7.3 Optical Sectioning and Imaging Resolution 223
7.4 Direct Detection of Multiphoton Absorption 228
7.5 Fluorescence Detection of Multiphoton Absorption 232
Bibliography 241
8 Pump-Probe Microscopy 245
8.1 Introduction 245
8.2 Pump-Probe Signals in Microscopy 246
8.3 Electronic Pump-Probe Spectroscopy 250
8.4 Detection of Pump-Probe Signals 264
8.5 Imaging Based on the Photothermal Effect 269
Bibliography 277
9 Harmonic Generation Microscopy 281
9.1 Introduction 281
9.2 Molecular Response in Harmonic Imaging 282
9.3 SHG Imaging of Fibrillar Structures 292
9.4 THG Imaging of ?(3) Discontinuities 304
Bibliography 310
10 Sum-Frequency Generation Microscopy 313
10.1 Introduction 313
10.2 Molecular Vibrations 314
10.3 Molecular Vibrations in Sum-Frequency Generation 324
10.4 Collinear Sum-Frequency Generation Microscopy 334
10.5 Third-Order Sum-Frequency Generation Microscopy 344
Bibliography 348
11 Coherent Raman Scattering Microscopy 351
11.1 Introduction 351
11.2 The Raman Effect 353
11.3 Coherent Raman Scattering 359
11.4 Raman Spectroscopy of Lipids 373
11.5 Imaging Properties of CARS 378
11.6 Imaging Properties of SRS 387
11.7 Spectral Resolution 391
Bibliography 398
Appendix A Fourier Transform Relationships 401
Appendix B Wavenumbers Unit 403
Appendix C Power Spectral Density of White Noise 405
Appendix D Fermi's Golden Rule 407
Appendix E Population Dynamics with Relaxation 411
Appendix F Stimulated Raman Scattering with Quantized Fields 413
Index 415
Acknowledgments xv
1 Light: Electromagnetic Radiation 1
1.1 Introduction 1
1.2 Electromagnetic Fields 1
1.3 Transverse Waves 7
1.4 Polarization States 15
1.5 Reflection and Transmission at Interfaces 19
1.6 Transformation of the Field by a Lens 23
1.7 Intensity and Energy 29
Bibliography 31
2 Focused Light 33
2.1 Introduction 33
2.2 Interference of Multiple Waves 34
2.3 The Scalar Focal Field 38
2.4 The Focused Vector Field 49
2.5 Aberrations 60
Bibliography 65
3 Ultrafast Pulses 67
3.1 Introduction 67
3.2 Optical Pulses in the Frequency Domain 68
3.3 Optical Pulses in the Time Domain 77
3.4 Measurement of Pulse Duration 88
3.5 Pulse Properties and Nonlinear Optical Signals 95
3.6 Noise 97
Bibliography 102
4 Classical Model of Nonlinear Optics 105
4.1 Introduction 105
4.2 Linear Optical Response 105
4.3 Nonlinear Optical Response 115
4.4 Properties of Nonlinear Susceptibilities 124
Bibliography 134
5 Semiclassical Model of Nonlinear Optics 137
5.1 Introduction 137
5.2 Quantum Mechanical Concepts 138
5.3 Density Matrix Formalism 147
5.4 Perturbation Expansion for the Density Matrix 152
5.5 Linear and Nonlinear Susceptibilities 159
5.6 Quantization of the Electromagnetic Field 164
Bibliography 172
6 Nonlinear Optical Signals: Molecular Transitions, Signal Radiation, Propagation, and Detection 175
6.1 Introduction 175
6.2 Molecular Transitions 175
6.3 Spatial Properties of Radiated Signal 187
6.4 Signal Radiation and Detection 205
Bibliography 211
7 Multiphoton Absorption and Fluorescence Microscopy 213
7.1 Introduction 213
7.2 Physics of Nonlinear Absorption 214
7.3 Optical Sectioning and Imaging Resolution 223
7.4 Direct Detection of Multiphoton Absorption 228
7.5 Fluorescence Detection of Multiphoton Absorption 232
Bibliography 241
8 Pump-Probe Microscopy 245
8.1 Introduction 245
8.2 Pump-Probe Signals in Microscopy 246
8.3 Electronic Pump-Probe Spectroscopy 250
8.4 Detection of Pump-Probe Signals 264
8.5 Imaging Based on the Photothermal Effect 269
Bibliography 277
9 Harmonic Generation Microscopy 281
9.1 Introduction 281
9.2 Molecular Response in Harmonic Imaging 282
9.3 SHG Imaging of Fibrillar Structures 292
9.4 THG Imaging of ?(3) Discontinuities 304
Bibliography 310
10 Sum-Frequency Generation Microscopy 313
10.1 Introduction 313
10.2 Molecular Vibrations 314
10.3 Molecular Vibrations in Sum-Frequency Generation 324
10.4 Collinear Sum-Frequency Generation Microscopy 334
10.5 Third-Order Sum-Frequency Generation Microscopy 344
Bibliography 348
11 Coherent Raman Scattering Microscopy 351
11.1 Introduction 351
11.2 The Raman Effect 353
11.3 Coherent Raman Scattering 359
11.4 Raman Spectroscopy of Lipids 373
11.5 Imaging Properties of CARS 378
11.6 Imaging Properties of SRS 387
11.7 Spectral Resolution 391
Bibliography 398
Appendix A Fourier Transform Relationships 401
Appendix B Wavenumbers Unit 403
Appendix C Power Spectral Density of White Noise 405
Appendix D Fermi's Golden Rule 407
Appendix E Population Dynamics with Relaxation 411
Appendix F Stimulated Raman Scattering with Quantized Fields 413
Index 415
Este título pertence ao(s) assunto(s) indicados(s). Para ver outros títulos clique no assunto desejado.
